Measurement of Second Hyperpolarizability and Nuclear Rotational Response of Gas-phase Carbon Disulfide
نویسندگان
چکیده
We use nonlinear beam deflection to separate the bound-electronic and nuclearrotational responses in gas-phase CS2. This allows a direct comparison of the second hyperpolarizability to our liquid CS2 measurements considering local-field effects. OCIS codes: (190.0190) Nonlinear optics, (190.3270) Kerr effect, (190.5650) Raman effect, (350.3250) Isotope separation
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